Defrost the Puff Pastry
Defrost overnight in the refrigerator or leave packaged at room temperature for about 40 minutes. For quicker thawing, remove one sheet, wrap in a paper towel, and microwave 15 seconds per side.
Mix the Sugar and Cinnamon
In a medium bowl, combine the granulated sugar and cinnamon thoroughly.
Roll Out the Puff Pastry
Unfold one defrosted sheet onto parchment paper. Roll gently in both directions to create a slightly thinner, even surface.
Add the Cinnamon Sugar Mixture
Sprinkle ¼ cup of the cinnamon sugar evenly over the surface. Roll lightly with a rolling pin so it adheres. Flip and repeat on the other side. Roll into approximately a 13” x 13” square.
Fold the Pastry
Fold each side inward toward the center twice, then fold one half over the other to form a book shape with six layers. Repeat with the second sheet.
Refrigerate
Chill the folded dough for 15 minutes to firm up.
Preheat Oven
Heat oven to 400°F (204°C).
Slice
Cut into ⅜-inch slices, yielding about 24 cookies per sheet.
Coat
Dip both sides into remaining cinnamon sugar. Place cut-side up, 2 inches apart on parchment-lined baking sheets. Slightly separate tops for a heart shape if desired.
Bake
Bake one tray at a time for 12 minutes. Flip and bake another 3–7 minutes until golden and caramelized. Watch carefully to prevent burning.
Cool
Transfer immediately to a wire rack. Cookies will crisp up as they cool. French Palmier Cookies should be crunchy and deeply caramelized.